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1.
Sci Total Environ ; 883: 163452, 2023 Jul 20.
Artigo em Inglês | MEDLINE | ID: mdl-37088383

RESUMO

Establishing mineral dust impacts on Earth's systems requires numerical models of the dust cycle. Differences between dust optical depth (DOD) measurements and modelling the cycle of dust emission, atmospheric transport, and deposition of dust indicate large model uncertainty due partially to unrealistic model assumptions about dust emission frequency. Calibrating dust cycle models to DOD measurements typically in North Africa, are routinely used to reduce dust model magnitude. This calibration forces modelled dust emissions to match atmospheric DOD but may hide the correct magnitude and frequency of dust emission events at source, compensating biases in other modelled processes of the dust cycle. Therefore, it is essential to improve physically based dust emission modules. Here we use a global collation of satellite observations from previous studies of dust emission point source (DPS) dichotomous frequency data. We show that these DPS data have little-to-no relation with MODIS DOD frequency. We calibrate the albedo-based dust emission model using the frequency distribution of those DPS data. The global dust emission uncertainty constrained by DPS data (±3.8 kg m-2 y-1) provides a benchmark for dust emission model development. Our calibrated model results reveal much less global dust emission (29.1 ± 14.9 Tg y-1) than previous estimates, and show seasonally shifting dust emission predominance within and between hemispheres, as opposed to a persistent North African dust emission primacy widely interpreted from DOD measurements. Earth's largest dust emissions, proceed seasonally from East Asian deserts in boreal spring, to Middle Eastern and North African deserts in boreal summer and then Australian shrublands in boreal autumn-winter. This new analysis of dust emissions, from global sources of varying geochemical properties, have far-reaching implications for current and future dust-climate effects. For more reliable coupled representation of dust-climate projections, our findings suggest the need to re-evaluate dust cycle modelling and benefit from the albedo-based parameterisation.

3.
Environ Sci Technol ; 46(19): 10390-404, 2012 Oct 02.
Artigo em Inglês | MEDLINE | ID: mdl-22994868

RESUMO

This paper reviews our knowledge of the measurement and modeling of mineral dust emissions to the atmosphere, its transport and deposition to the ocean, the release of iron from the dust into seawater, and the possible impact of that nutrient on marine biogeochemistry and climate. Of particular concern is our poor understanding of the mechanisms and quantities of dust deposition as well as the extent of iron solubilization from the dust once it enters the ocean. Model estimates of dust deposition in remote oceanic regions vary by more than a factor of 10. The fraction of the iron in dust that is available for use by marine phytoplankton is still highly uncertain. There is an urgent need for a long-term marine atmospheric surface measurement network, spread across all oceans. Because the southern ocean is characterized by large areas with high nitrate but low chlorophyll surface concentrations, that region is particularly sensitive to the input of dust and iron. Data from this region would be valuable, particularly at sites downwind from known dust source areas in South America, Australia, and South Africa. Coordinated field experiments involving both atmospheric and marine measurements are recommended to address the complex and interlinked processes and role of dust/Fe fertilization on marine biogeochemistry and climate.


Assuntos
Atmosfera , Poeira , Minerais , Oceanos e Mares , Atmosfera/química , Austrália , Clorofila , Poeira/análise , Ferro/química , Biologia Marinha/métodos , Modelos Teóricos , Pesquisa/tendências , Água do Mar/química , África do Sul
4.
Proc Natl Acad Sci U S A ; 106(49): 20564-71, 2009 Dec 08.
Artigo em Inglês | MEDLINE | ID: mdl-19620716

RESUMO

Dust plays a vital role in climate and biophysical feedbacks in the Earth system. One source of dust, the Bodélé Depression in Chad, is estimated to produce about half the mineral aerosols emitted from the Sahara, which is the world's largest source. By using a variety of new remote sensing data, regional modeling, trajectory models, chemical analyses of dust, and future climate simulations, we investigate the current and past sensitivity of the Bodélé. We show that minor adjustments to small features of the atmospheric circulation, such as the Bodélé Low-Level Jet, could profoundly alter the behavior of this feature. Dust production during the mid-Holocene ceased completely from this key source region. Although subject to a great deal of uncertainty, some simulations of the 21st century indicate the potential for a substantial increase in dust production by the end of the century in comparison with current values.

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